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Cu(In 4

Ga)Se₂ 3

光催化 3

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PM10sub> emissions from industrial coal-fired chain-grate boilers

Xinghua Li, Junzan Han, Lei Duan

《环境科学与工程前沿（英文）》 2017年第11卷第6期 doi: 10.1007/s11783-017-0966-y

摘要： Industrial coal-fired boiler is an important air pollutant emission source in China. The chain-grate boiler is the most extensively used type of industrial coal-fired boiler. An electrical low-pressure impactor, and a Dekati Low Pressure Impactor were applied to determine mass and number size distributions of PM at the inlet and the outlet of the particulate emission control devices at six coal-fired chain-grate boilers. The mass size distribution of PM generated from coal-fired chain-grate boilers generally displays a bimodal distribution that contains a submicron mode and a coarse mode. The PM in the submicron mode for burning with raw coal contributes to 33%±10 % of PM emissions, much higher than those for pulverized boilers. And the PM in the submicron mode for burning with briquette contributes up to 86 % of PM emissions. Multiclones and scrubbers are not efficient for controlling PM emission. Their average collection efficiencies for sub-micron particle and super-micron particle are 34% and 78%, respectively. Operating conditions of industrial steam boilers have influence on PM generation. Peak of the submicron mode during normal operation period is larger than the start-up period.

关键词： coal-fired chain-grate boiler PM₁₀ size distribution particulate emission control devices size-dependent collection efficiency

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大气悬浮颗粒PM10sub>对感烟火灾探测器本底效应研究

谢启源,袁宏永,蒋亚龙

《中国工程科学》 2003年第5卷第6期页码 84-87

摘要：

针对大气污染引起的悬浮颗粒,尤其是可吸入颗粒（PM10sub>）对感烟火灾探测器产生的本底效应进行了分析，并以离子型感烟探测器为例对本底值进行计算，通过比较，显示不同程度的大气颗粒物污染对感烟探测器本底影响的差异极小

关键词：悬浮颗粒火灾探测本底效应

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Airborne bacteria associated with particulate matter from a highly urbanised metropolis: A potential risk to the population’s health

《环境科学与工程前沿（英文）》 2022年第16卷第9期 doi: 10.1007/s11783-022-1552-5

摘要：

• The airborne bacteria of Mexico City are representative of urban environments.

关键词： Airborne bacteria Urbanisation PM₁₀ Mexico City Microbiome

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一种融合多特征聚类与神经网络的PM2.5sub>小时浓度预测新模型及其在中国城市的应用 Article

刘辉, 龙治豪, 段铸, 施惠鹏

《工程（英文）》 2020年第6卷第8期页码 944-956 doi: 10.1016/j.eng.2020.05.009

摘要：

PM2.5sub>浓度预测对空气污染物早期预警具有重要意义。本文提出一种改进的PM2.5sub>浓度多步预测模型，即多特征聚类分解(MCD)-回声状态网络(ESN)-粒子群优化(PSO)混合模型。该模型包括分解预测部分和优化预测部分。在MCD方法中，采用RSAR算法选择重要的空气污染物变量，使用KC算法对所得变量进行聚类，利用EWT算法将PM2.5sub>浓度序列的聚类结果分解为多个子层。利用我国4个不同城市的真实PM2.5sub>浓度数据，验证了所提出模型的有效性。实验结果表明，所提出预测模型适用于PM2.5sub>浓度的多步高精度预测，具有比基准模型更优的预测性能。

关键词： PM2.5sub>2.5浓度预测 PM2.5sub>2.5浓度聚类经验小波分解多步预测

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An assessment of the potential health benefits of realizing the goals for PM

Guoxia MA,Jinnan WANG,Fang YU,Yanshen ZHANG,Dong CAO

《环境科学与工程前沿（英文）》 2016年第10卷第2期页码 288-298 doi: 10.1007/s11783-014-0738-x

摘要： As a response to the severe air quality problems in China, the Chinese Ministry of Environmental Protection in 2012 issued an updated (GB3095-2012), which set a stricter grade II PM standard. A successful implementation of this standard will have an impact on human health through reduction of exposure to air pollution in the population. Using the methods of adjusted human capital and value of statistical life, the authors in this article estimate the economic impact of a successful implementation of the updated on human health in China. The key results are: 1) The human health benefits from reaching the updated standard for PM would equal CNY 51.1 billion using adjusted human capital, accounting for 18.5% of total human health costs in China, and CNY 83.5 billion using the value of a statistical life; 2) the benefit of reaching the updated standard for PM is highest in the east coastal areas and gradually declines for more Western provinces; and 3) the marginal benefit of public health increases as the environmental quality standard PM improves. If the annual concentration of PM were to be reduced from the target number in the original grade II standard to that in the updated standard, the mortality rate of long-term exposure would be reduced by 6.5% due to reduced chronic exposure. In addition, if the annual concentration were to be reduced further from updated grade II to grade I standard, the mortality rate for long-term exposure would be lowered by 32.8%.

关键词： air quality health benefit Ambient Air Quality Standard PM₁₀ China

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Diverse bacterial populations of PM in urban and suburb Shanghai, China

《环境科学与工程前沿（英文）》 2021年第15卷第3期 doi: 10.1007/s11783-020-1329-7

摘要：

• Urban aerosols harbour diverse bacterial communities in Shanghai.

关键词： PM_2.5 Bacteria 16S rRNA SEM analysis Shanghai City

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Temporal variation of PM-associated health effects in Shijiazhuang, Hebei

《环境科学与工程前沿（英文）》 2021年第15卷第5期 doi: 10.1007/s11783-020-1376-0

摘要：

•Annual mean PM_2.5 in Shijiazhuang were 87, 95, and 82 µg/m³ in 2015–2017.

关键词： PM_2.5 Health effects Integrated exposure-response model Shijiazhuang

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Real drive cycles analysis by ordered power methodology applied to fuel consumption, CO

Pol Masclans Abelló, Vicente Medina Iglesias, M. Antonia de los Santos López, Jesús Álvarez-Flórez

《环境科学与工程前沿（英文）》 2021年第15卷第1期 doi: 10.1007/s11783-020-1296-z

摘要： Abstract • New method named CAbOP is presented based on ordering data according to power. • Three emission models are used and their emission results compared. • Emissions data are analyzed in real driving cycles under CAbOP criteria. • Methodology to collect data and reconstruct lost data in real urban driving cycles. In this work three fuel consumption and exhaust emission models, ADVISOR, VT-MICRO and the European Environmental Agency Emission factors, have been used to obtain fuel consumption (FC) and exhaust emissions. These models have been used at micro-scale, using the two signal treatment methods presented. The manuscript presents: 1) a methodology to collect data in real urban driving cycles, 2) an estimation of FC and tailpipe emissions using some available models in literature, and 3) a novel analysis of the results based on delivered wheel power. The results include Fuel Consumption (FC), CO2, NOx and PM10 emissions, which are derived from the three simulators. In the first part of the paper we present a new procedure for incomplete drive cycle data treatment, which is necessary for real drive cycle acquisition in high density cities. Then the models are used to obtain second by second FC and exhaust emissions. Finally, a new methodology named Cycle Analysis by Ordered Power (CAbOP) is presented and used to compare the results. This method consists in the re-ordering of time dependant data, considering the wheel mechanical power domain instead of the standard time domain. This new strategy allows the 5 situations in drive cycles to be clearly visualized: hard breaking zone, slowdowns, idle or stop zone, sustained speed zone and acceleration zone. The complete methodology is applied in two real drive cycles surveyed in Barcelona (Spain) and the results are compared with a standardized WLTC urban cycle.

关键词： Cycle Analysis by Ordered Power (CAbOP) Micro and macro models Real drive cycle NO_x/PM₁₀/CO₂ emissions Wheel mechanical power domain Worldwide Harmonized Light-Duty Vehicles Test Cycle (WLTC)

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Local and regional contributions to PM in the Beijing 2022 Winter Olympics infrastructure areas during

《环境科学与工程前沿（英文）》 2021年第15卷第6期 doi: 10.1007/s11783-021-1434-2

摘要：

• Regional transportation contributed more than local emissions during haze episodes.

关键词： 2022 Winter Olympics PM_2.5 Source apportionment

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PM concentration declining saves health expenditure in China

《环境科学与工程前沿（英文）》 2023年第17卷第7期 doi: 10.1007/s11783-023-1690-4

摘要：

● Monthly hospitalization expenses are sensitive to increases in PM_2.5 exposure.

关键词： Air pollution Health expenditure PM_2.5 concentration Economic impact Heterogeneous effect

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PM2.5 over North China based on MODIS AOD and effect of meteorological elements during 2003‒2015

Youfang Chen, Yimin Zhou, Xinyi Zhao

《环境科学与工程前沿（英文）》 2020年第14卷第2期 doi: 10.1007/s11783-019-1202-8

摘要： The Taihang Mountains was the boundary between high and low pollution areas. There were one high value center for PM2.5 pollution and two low value centers. In 2004, 2009 and after 2013, PM2.5 concentration was relatively low. Over the past 40 years, PM2.5 pollution in North China has become increasingly serious and progressively exposes the densely populated areas to pollutants. However, due to limited ground data, it is challenging to estimate accurate PM2.5 exposure levels, further making it unfavorable for the prediction and prevention of PM2.5 pollutions. This paper therefore uses the mixed effect model to estimate daily PM2.5 concentrations of North China between 2003 and 2015 with ground observation data and MODIS AOD satellite data. The tempo-spatial characteristics of PM2.5 and the influence of meteorological elements on PM2.5 is discussed with EOF and canonical correlation analysis respectively. Results show that overall R2 is 0.36 and the root mean squared predicted error was 30.1 μg/m3 for the model prediction. Our time series analysis showed that, the Taihang Mountains acted as a boundary between the high and low pollution areas in North China; while the northern part of Henan Province, the southern part of Hebei Province and the western part of Shandong Province were the most polluted areas. Although, in 2004, 2009 and dates after 2013, PM2.5 concentrations were relatively low. Meteorological/topography conditions, that include high surface humidity of area in the range of 34°‒40°N and 119°‒124°E, relatively low boundary layer heights, and southerly and easterly winds from the east and north area were common factors attributed to haze in the most polluted area. Overall, the spatial distribution of increasingly concentrated PM2.5 pollution in North China are consistent with the local emission level, unfavorable meteorological conditions and topographic changes.

关键词： Aerosol optical depth PM_2.5 MODIS Mixed effect model Canonical correlation analysis

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我国一次气溶胶和二次无机气溶胶大气年龄的时空分布特征 Article

Xiaodong Xie, Qi Ying, 张宏亮, 胡建林

《工程（英文）》 2023年第28卷第9期页码 117-129 doi: 10.1016/j.eng.2022.03.013

摘要：本研究使用年龄可分辨的社区多尺度空气质量模型CMAQ对我国一次和二次无机细颗粒物（PM2.5sub>）的年龄分布进行了为期一年的模拟。结果表明，一次PM2.5sub>（PPM）和铵盐主要来源于本地的新鲜排放，我国大部分地区约60%~80%集中在0~24 h年龄档。本研究中基于年龄可分辨的CMAQ模型得到的PM2.5sub>年龄信息可以帮助政府部分制定有效的应急排放控制措施，有助于消除重污染天气。

关键词：大气年龄 PM2.5sub> CMAQ模型控制措施

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NO hydrogenation to NH over FeCu/TiO catalyst with improved activity

《化学科学与工程前沿（英文）》 2023年第17卷第12期页码 1973-1985 doi: 10.1007/s11705-023-2364-2

摘要： Ammonia is crucial in industry and agriculture, but its production is hindered by environmental concerns and energy-intensive processes. Hence, developing an efficient and environmentally friendly catalyst is imperative. In this study, we employed a straightforward and efficient impregnation technique to create various Cu-doped catalysts. Notably, the optimized 10Fe-8Cu/TiO₂ catalyst exhibited exceptional catalytic performance in converting NO to NH₃, achieving an NO conversion rate exceeding 80% and an NH₃ selectivity exceeding 98% at atmospheric pressure and 350 °C. We employed in situ diffuse reflectance Fourier transform infrared spectroscopy and conducted density functional theory calculations to investigate the intermediates and subsequent adsorption. Our findings unequivocally demonstrate that Cu doping enhances the rate-limiting hydrogenation step and lowers the energy barrier for NH₃ desorption, thereby resulting in improved NO conversion and enhanced selectivity toward ammonia. This study presents a pioneering approach toward energy-efficient ammonia synthesis and recycling of nitrogen sources.

关键词： NO hydrogenation synthetic ammonia 10Fe-xCu/TiO₂ high selectivity

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Does environmental infrastructure investment contribute to emissions reduction? A case of China

Xiaoqian SONG, Yong GENG, Ke LI, Xi ZHANG, Fei WU, Hengyu PAN, Yiqing ZHANG

《能源前沿（英文）》 2020年第14卷第1期页码 57-70 doi: 10.1007/s11708-019-0654-7

摘要： Environmental infrastructure investment (EII) is an important environmental policy instrument on responding to greenhouse gas (GHG) emission and air pollution. This paper employs an improved stochastic impact by regression on population, affluence and technology (STRIPAT) model by using panel data from 30 Chinese provinces and municipalities for the period of 2003–2015 to investigate the effect of EII on CO emissions, SO emissions, and PM pollution. The results indicate that EII has a positive and significant effect on mitigating CO emission. However, the effect of EII on SO emission fluctuated although it still contributes to the reduction of PM pollution through technology innovations. Energy intensity has the largest impact on GHG emissions and air pollution, followed by GDP per capita and industrial structure. In addition, the effect of EII on environmental issues varies in different regions. Such findings suggest that policies on EII should be region-specific so that more appropriate mitigation policies can be raised by considering the local realities.

关键词： environmental infrastructure investment (EII) CO₂ emission SO₂ emission PM_2.5 pollution stochastic impact by regression on population affluence and technology (STIRPAT) model governance

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Spatial and Temporal Distribution of PM

Xiao-hong Chen,Xiang-bo Tang

《工程管理前沿（英文）》 2016年第3卷第2期页码 171-181 doi: 10.15302/J-FEM-2016017

摘要： Utilizing the initial hourly monitoring data of PM concentrations at 23 monitoring sites across the Chang-Zhu-Tan city cluster between January 2013 and February 2014 that released in Real-time Air Quality Reporting System in Hunan Province, this paper draws diagrams and analyzes the change rule of the pollutants concentration over time. In addition, this paper studies the regional distribution of PM seasonal pollution in the vicinity of the monitoring sites using ArcGIS geographic information system with the Kriging interpolation method. On this basis, this paper puts forward some effective control strategies to cope with regional PM pollution combined with the information of industry distribution and development status in the Chang-Zhu-Tan city cluster.

关键词： PM_2.5 spatial and temporal distribution ArcGIS the chang-Zhu-Tan city cluster